I have "Green Onions" by Booker T. & The M.G.'s on my cell. It never fails to elicit smiles when it plays in public. Wicked guitar playing by Steve Cropper.
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The Maryland Pacesetters Steelband Orchestra has a cover of Marvin Gaye’s “Sexual Healing” that I use on my phone. Distinctive, easy to hear in a crowd, and usually elicits a smile once people figure out what they are listening to.