I use iTunes I also use excel for inventory lists.
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I probably should have mentioned...I was also looking for fast and easy data entry. The software allows the use of a barcode scanner..zippp..and everything is in there.
My excel spreadsheets at work often exceed excel's maximum 66000+ rows (I shift over to access at that point), but I didn't want to type in the various CD data fields.
I use Collectorz.com Music Collector. It allows you to use a bar-code scanner or searches various databases directly from the CD. It also offers an app for the iPhone that allows you sync your desktop database to your iPhone - very handy when shopping to avoid duplicates.