I have a Vault 2 and I don’t know, but my guess is you have to do it through a PC or Mac with the Vault being on your network. Pretty sure you can’t do it through your phone or an iPad/tablet which is all I use. I’ve only copied one CD twice so I’ll be interested in someone responding how to do this too.
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Google is your friend. When I did a search on "Bluesound Vault 2 delete album" it says you have to do it from a computer on the same network. It linked to this article: